Voltammetric and impedance studies of phenols and its derivatives at carbon nanotubes/Prussian blue films platinum modified electrode

A. S. Adekunle, O. A. Arotiba, B. O. Agboola, N. W. Maxakato, B. B. Mamba, E. E. Ebenso

Research output: Chapter in Book/Report/Conference proceedingConference contributionpeer-review

Abstract

The electrochemical oxidation of phenol (Ph), 4-chlorophenol (4-ClPh) and 4-nitrophenol (4-NPh) at a platinum electrode modified with and without multi-walled carbon nanotubes/Prussian blue nanocomposite was investigated by cyclic voltammetry (CV) and impedance measurements. The modified electrodes were characterized using transmission electron microscopy (TEM), electron X-ray dispersive spectroscopy (XRD), cyclic voltammetry (CVs) and electrochemical impedance spectroscopy (EIS). Pt-MWCNT-PB electrode gave the highest electrooxidation current compared to the other electrodes studied. The oxidation of the phenol was characterized by some level of adsorption. The degree of adsorption was depicted by theTafel values of 4292.4, 663.2 and 203.8 mVdec -1 for Ph, 4-ClPh and 4-NPh respectively. The limits of detection were in the micro molar range and the Gibbs free energy change (ΔG°) due to adsorption was estimated as -33.8, -35.8 and -36.0 kJmol-1 for Ph, 4-ClPh and 4-NPh.

Original languageEnglish
Title of host publicationTechnical Proceedings of the 2014 NSTI Nanotechnology Conference and Expo, NSTI-Nanotech 2014
PublisherNano Science and Technology Institute
Pages280-283
Number of pages4
ISBN (Print)9781482258301
Publication statusPublished - 2014
EventNanotechnology 2014: Electronics, Manufacturing, Environment, Energy and Water - 2014 NSTI Nanotechnology Conference and Expo, NSTI-Nanotech 2014 - Washington, DC, United States
Duration: 15 Jun 201418 Jun 2014

Publication series

NameTechnical Proceedings of the 2014 NSTI Nanotechnology Conference and Expo, NSTI-Nanotech 2014
Volume3

Conference

ConferenceNanotechnology 2014: Electronics, Manufacturing, Environment, Energy and Water - 2014 NSTI Nanotechnology Conference and Expo, NSTI-Nanotech 2014
Country/TerritoryUnited States
CityWashington, DC
Period15/06/1418/06/14

Keywords

  • Adsorption
  • Impedance measurement
  • Phenols
  • Platinum electrode
  • Prussian blue nanoparticles

ASJC Scopus subject areas

  • Hardware and Architecture
  • Electrical and Electronic Engineering
  • Electronic, Optical and Magnetic Materials

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