Topological magnon insulator spin excitations in the two-dimensional ferromagnet CrBr3

Topological magnons are bosonic analogues of topological fermions in electronic systems. They have been studied extensively by theory but rarely realized by experiment. Here, by performing inelastic neutron scattering measurements on single crystals of a two-dimensional ferromagnet CrBr3, which was classified as Dirac magnon semimetal featured by the linear bands crossing at the Dirac points, we fully map out the magnetic excitation spectra, and reveal that there is an apparent gap of ∼3.5 meV between the acoustic and optical branches of the magnons at the K point. By collaborative efforts between experiment and theoretical calculations using a five-orbital Hubbard model obtained from first-principles calculations to derive the exchange parameters, we find that a Hamiltonian with Heisenberg exchange interactions, next-nearest-neighbor Dzyaloshinskii-Moriya (DM) interaction, and single-ion anisotropy is more appropriate to describe the system. Calculations using the model show that the lower and upper magnon bands separated by the gap exhibit Chern numbers of ±1. These results indicate that CrBr3 is a topological magnon insulator, where the nontrivial gap is a result of the DM interaction.