Spin fluctuations in Sr1.8La0.2RuO4

  • Zheng He
  • , Qisi Wang
  • , Yu Feng
  • , Chul Kim
  • , Wonshik Kyung
  • , Changyoung Kim
  • , Hongliang Wo
  • , Gaofeng Ding
  • , Yiqing Hao
  • , Feiyang Liu
  • , Helen C. Walker
  • , Devashibhai T. Adroja
  • , Astrid Schneidewind
  • , Wenbin Wang
  • , Jun Zhao

Research output: Contribution to journalArticlepeer-review

1 Citation (Scopus)

Abstract

We use inelastic neutron scattering to study spin fluctuations in Sr1.8La0.2RuO4, where Lanthanum doping triggers a Lifshitz transition by pushing the van Hove singularity in the γ band to the Fermi energy. Strong spin fluctuations emerge at an incommensurate wave vector Qic=(0.3,0.3), corresponding to the nesting vector between α and β Fermi sheets. The incommensurate antiferromagnetic fluctuations shift toward (0.25,0.25) with increasing energy up to ∼110 meV. By contrast, scatterings near the ferromagnetic wave vectors Q=(1,0) and (1,1) remain featureless at all energies. This contradicts the weak-coupling perspective that suggests a sharp enhancement of ferromagnetic susceptibility due to the divergence of density of states in the associated γ band. Our findings imply that ferromagnetic fluctuations in Sr2RuO4 and related materials do not fit into the weak-coupling paradigm, but instead are quasilocal fluctuations induced by Hund's coupling. This imposes significant constraints for the pairing mechanism involving spin fluctuations.

Original languageEnglish
Article numberL201107
JournalPhysical Review B
Volume107
Issue number20
DOIs
Publication statusPublished - 15 May 2023

ASJC Scopus subject areas

  • Electronic, Optical and Magnetic Materials
  • Condensed Matter Physics

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