Spin fluctuations in Sr1.8La0.2RuO4

Zheng He, Qisi Wang, Yu Feng, Chul Kim, Wonshik Kyung, Changyoung Kim, Hongliang Wo, Gaofeng Ding, Yiqing Hao, Feiyang Liu, Helen C. Walker, Devashibhai T. Adroja, Astrid Schneidewind, Wenbin Wang, Jun Zhao

Research output: Contribution to journalArticlepeer-review

Abstract

We use inelastic neutron scattering to study spin fluctuations in Sr1.8La0.2RuO4, where Lanthanum doping triggers a Lifshitz transition by pushing the van Hove singularity in the γ band to the Fermi energy. Strong spin fluctuations emerge at an incommensurate wave vector Qic=(0.3,0.3), corresponding to the nesting vector between α and β Fermi sheets. The incommensurate antiferromagnetic fluctuations shift toward (0.25,0.25) with increasing energy up to ∼110 meV. By contrast, scatterings near the ferromagnetic wave vectors Q=(1,0) and (1,1) remain featureless at all energies. This contradicts the weak-coupling perspective that suggests a sharp enhancement of ferromagnetic susceptibility due to the divergence of density of states in the associated γ band. Our findings imply that ferromagnetic fluctuations in Sr2RuO4 and related materials do not fit into the weak-coupling paradigm, but instead are quasilocal fluctuations induced by Hund's coupling. This imposes significant constraints for the pairing mechanism involving spin fluctuations.

Original languageEnglish
Article numberL201107
JournalPhysical Review B
Volume107
Issue number20
DOIs
Publication statusPublished - 15 May 2023

ASJC Scopus subject areas

  • Electronic, Optical and Magnetic Materials
  • Condensed Matter Physics

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