Second harmonic scattering from mass characterized 2D graphene oxide sheets

Isabelle Russier-Antoine; Hussein Fakhouri; Srestha Basu; Franck Bertorelle; Philippe Dugourd; Pierre François Brevet; Prajitha Velayudhan; Sabu Thomas; Nandakumar Kalarikkal; Rodolphe Antoine

doi:10.1039/d0cc00111b

Second harmonic scattering from mass characterized 2D graphene oxide sheets

Isabelle Russier-Antoine
, Hussein Fakhouri
, Srestha Basu
, Franck Bertorelle
, Philippe Dugourd
, Pierre François Brevet
, Prajitha Velayudhan
, Sabu Thomas
, Nandakumar Kalarikkal
, Rodolphe Antoine

Research output: Contribution to journal › Article › peer-review

23 Citations (Scopus)

Abstract

In this communication, we report the second harmonic scattering from mass characterized 2D graphene oxide sheets dispersed in an aqueous suspension, in the femtosecond regime at 800 nm laser excitation. Charge-detection mass-spectrometry, performing at the single sheet level, allows for an exhaustive molar mass distribution and thus concentration for these 2D nanomaterials samples. The orientation-averaged hyperpolarizability value is (1.36 ± 0.15) × 10^-25 esu as determined by the concentration-dependent harmonic scattering signal. In addition, the multi-photon excited fluorescence spectrum is characterized by a broad band in the visible range between 350 and 700 nm centered at about 500 nm.

Original language	English
Pages (from-to)	3859-3862
Number of pages	4
Journal	Chemical Communications
Volume	56
Issue number	27
DOIs	https://doi.org/10.1039/d0cc00111b
Publication status	Published - 7 Apr 2020
Externally published	Yes

ASJC Scopus subject areas

Electronic, Optical and Magnetic Materials
Catalysis
Ceramics and Composites
General Chemistry
Surfaces, Coatings and Films
Metals and Alloys
Materials Chemistry

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10.1039/d0cc00111b

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title = "Second harmonic scattering from mass characterized 2D graphene oxide sheets",

abstract = "In this communication, we report the second harmonic scattering from mass characterized 2D graphene oxide sheets dispersed in an aqueous suspension, in the femtosecond regime at 800 nm laser excitation. Charge-detection mass-spectrometry, performing at the single sheet level, allows for an exhaustive molar mass distribution and thus concentration for these 2D nanomaterials samples. The orientation-averaged hyperpolarizability value is (1.36 ± 0.15) × 10-25 esu as determined by the concentration-dependent harmonic scattering signal. In addition, the multi-photon excited fluorescence spectrum is characterized by a broad band in the visible range between 350 and 700 nm centered at about 500 nm.",

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doi = "10.1039/d0cc00111b",

language = "English",

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AU - Russier-Antoine, Isabelle

AU - Fakhouri, Hussein

AU - Basu, Srestha

AU - Bertorelle, Franck

AU - Dugourd, Philippe

AU - Brevet, Pierre François

AU - Velayudhan, Prajitha

AU - Thomas, Sabu

AU - Kalarikkal, Nandakumar

AU - Antoine, Rodolphe

PY - 2020/4/7

Y1 - 2020/4/7

N2 - In this communication, we report the second harmonic scattering from mass characterized 2D graphene oxide sheets dispersed in an aqueous suspension, in the femtosecond regime at 800 nm laser excitation. Charge-detection mass-spectrometry, performing at the single sheet level, allows for an exhaustive molar mass distribution and thus concentration for these 2D nanomaterials samples. The orientation-averaged hyperpolarizability value is (1.36 ± 0.15) × 10-25 esu as determined by the concentration-dependent harmonic scattering signal. In addition, the multi-photon excited fluorescence spectrum is characterized by a broad band in the visible range between 350 and 700 nm centered at about 500 nm.

AB - In this communication, we report the second harmonic scattering from mass characterized 2D graphene oxide sheets dispersed in an aqueous suspension, in the femtosecond regime at 800 nm laser excitation. Charge-detection mass-spectrometry, performing at the single sheet level, allows for an exhaustive molar mass distribution and thus concentration for these 2D nanomaterials samples. The orientation-averaged hyperpolarizability value is (1.36 ± 0.15) × 10-25 esu as determined by the concentration-dependent harmonic scattering signal. In addition, the multi-photon excited fluorescence spectrum is characterized by a broad band in the visible range between 350 and 700 nm centered at about 500 nm.

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DO - 10.1039/d0cc00111b

M3 - Article

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VL - 56

SP - 3859

EP - 3862

JO - Chemical Communications

JF - Chemical Communications

IS - 27

ER -

Second harmonic scattering from mass characterized 2D graphene oxide sheets

Abstract

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