TY - JOUR
T1 - MOF-derived magnetic nanocomposites as potential formulations for the efficient removal of organic pollutants from water via adsorption and advanced oxidation processes
T2 - A review
AU - Miyah, Youssef
AU - El Messaoudi, Noureddine
AU - Benjelloun, Mohammed
AU - Georgin, Jordana
AU - Franco, Dison Stracke Pfingsten
AU - Acikbas, Yaser
AU - Kusuma, Heri Septya
AU - Sillanpää, Mika
N1 - Publisher Copyright:
© 2024 Elsevier Ltd
PY - 2024/12
Y1 - 2024/12
N2 - This review article summarizes current developments in the design and application of metal-organic framework (MOF)-derived magnetic nanocomposites (MNCs) to remove organic pollutants (OPs) in water efficiently. In the review, various methods for synthesis, like in-situ encapsulation and post-synthetic modification, have been discussed, showing how magnetic nanoparticles incorporated into MOFs resulted in materials that had improved adsorption and advanced oxidation processes. These NCs showed unique structural characteristics and functional advantages given their large surface area, tunable pore sizes, and magnetic separability. This work has emphasized dual functionality concerning adsorption and photocatalytic degradation. More importantly, these processes synergistically cooperate to realize considerably high removal efficiencies for a wide range of OPs. It also addresses current challenges on stability and scalability issues and proposes possible ways of improving MOF-MNCs' performance. This is followed by future research directions on the betterment of the practical application of MOF-MNCs in controlling water pollution, highlighting their potential as a feasible and effective solution for mitigating water contamination. Lastly, it is proposed in this synthesis that Ishikawa 5Ms should be considered when developing low-cost MOF-MNCs and industrializing their application for water depollution.
AB - This review article summarizes current developments in the design and application of metal-organic framework (MOF)-derived magnetic nanocomposites (MNCs) to remove organic pollutants (OPs) in water efficiently. In the review, various methods for synthesis, like in-situ encapsulation and post-synthetic modification, have been discussed, showing how magnetic nanoparticles incorporated into MOFs resulted in materials that had improved adsorption and advanced oxidation processes. These NCs showed unique structural characteristics and functional advantages given their large surface area, tunable pore sizes, and magnetic separability. This work has emphasized dual functionality concerning adsorption and photocatalytic degradation. More importantly, these processes synergistically cooperate to realize considerably high removal efficiencies for a wide range of OPs. It also addresses current challenges on stability and scalability issues and proposes possible ways of improving MOF-MNCs' performance. This is followed by future research directions on the betterment of the practical application of MOF-MNCs in controlling water pollution, highlighting their potential as a feasible and effective solution for mitigating water contamination. Lastly, it is proposed in this synthesis that Ishikawa 5Ms should be considered when developing low-cost MOF-MNCs and industrializing their application for water depollution.
KW - Adsorption
KW - Advanced oxidation process
KW - Cost
KW - MOF-Magnetic nanocomposites
KW - Organic pollutants
UR - http://www.scopus.com/inward/record.url?scp=85204560316&partnerID=8YFLogxK
U2 - 10.1016/j.mtsust.2024.100985
DO - 10.1016/j.mtsust.2024.100985
M3 - Review article
AN - SCOPUS:85204560316
SN - 2589-2347
VL - 28
JO - Materials Today Sustainability
JF - Materials Today Sustainability
M1 - 100985
ER -