TY - JOUR
T1 - Computational study of γ-ray and fast neutron shielding efficacy of (70–x)B2O3 – 5TeO2 – 20SrO – 5ZnO – (x)Bi2O3 glass systems using Phy-X/PSD, XCOM and GEANT-4
AU - Kheswa, Bonginkosi Vincent
AU - Makhathini, Lucky
AU - Majola, Siyabonga Ntokozo
N1 - Publisher Copyright:
© 2024 Walter de Gruyter GmbH. All rights reserved.
PY - 2024
Y1 - 2024
N2 - This study investigated the LAC, MAC, half-value thickness, tenth-value thickness, mean free path, Zeff, Neff, FNRCS, EBF, and EABF of a glass composition (70-x)B2O3 –5TeO2 – 20SrO – 5ZnO – (x)Bi2O3, with x ranging from 0 to 15 mol%. Sample S5 showed the lowest HVT, TVT, and MFP and the highest MAC, LAC, Zeff, and Neff across 300 keV–15 MeV, indicating enhanced γ-ray shielding with higher Bi2O3 content in narrow-beam applications. However, EBF and EABF decreased with Bi2O3 at 0.5 and 1 MeV, but increased at 10 MeV, indicating improved shielding only at low and intermediate energies in broad-beam scenarios. Sample S4 exhibited the highest FNRCS and best neutron shielding efficiency. The comparison of our results with the literature revealed that S5 and S4 are, respectively, even more superior, in shielding γ radiation and neutrons than some of the glass materials that have been recently investigated in the literature. Therefore, in γ-ray shielding applications, incorporating Bi2O3 into the glass matrix is advisable primarily for narrow-beam conditions, and for broad-beam scenarios at intermediate energies, but not at high energies in broad-beam contexts.
AB - This study investigated the LAC, MAC, half-value thickness, tenth-value thickness, mean free path, Zeff, Neff, FNRCS, EBF, and EABF of a glass composition (70-x)B2O3 –5TeO2 – 20SrO – 5ZnO – (x)Bi2O3, with x ranging from 0 to 15 mol%. Sample S5 showed the lowest HVT, TVT, and MFP and the highest MAC, LAC, Zeff, and Neff across 300 keV–15 MeV, indicating enhanced γ-ray shielding with higher Bi2O3 content in narrow-beam applications. However, EBF and EABF decreased with Bi2O3 at 0.5 and 1 MeV, but increased at 10 MeV, indicating improved shielding only at low and intermediate energies in broad-beam scenarios. Sample S4 exhibited the highest FNRCS and best neutron shielding efficiency. The comparison of our results with the literature revealed that S5 and S4 are, respectively, even more superior, in shielding γ radiation and neutrons than some of the glass materials that have been recently investigated in the literature. Therefore, in γ-ray shielding applications, incorporating Bi2O3 into the glass matrix is advisable primarily for narrow-beam conditions, and for broad-beam scenarios at intermediate energies, but not at high energies in broad-beam contexts.
KW - bismuth
KW - borate
KW - neutron
KW - shielding
KW - γ radiation
UR - http://www.scopus.com/inward/record.url?scp=85206312084&partnerID=8YFLogxK
U2 - 10.1515/ract-2024-0316
DO - 10.1515/ract-2024-0316
M3 - Article
AN - SCOPUS:85206312084
SN - 0033-8230
JO - Radiochimica Acta
JF - Radiochimica Acta
ER -