A μSR study of the valence phase transition in the double perovskites Ba2PrRu1-xIrxO6

A. D. Hillier; D. T. Adroja; W. Kockelmann; M. Wakeshima; Y. Izumiyama; Y. Hinatsu; D. Visser; B. D. Rainford

doi:10.1016/j.jmmm.2006.10.540

A μSR study of the valence phase transition in the double perovskites Ba₂PrRu_1-xIr_xO₆

A. D. Hillier, D. T. Adroja, W. Kockelmann, M. Wakeshima, Y. Izumiyama, Y. Hinatsu, D. Visser, B. D. Rainford

Research output: Contribution to journal › Article › peer-review

2 Citations (Scopus)

Abstract

The recent bulk studies have revealed the first-order valence phase transition in Ba₂PrRu_1-xIr_xO₆ (0.10≤x≤0.25), while the compounds with x=0 and 1 show antiferromagnetic ordering with T_N=120 and 71 K, respectively. We have carried out zero-field (ZF) muon spin relaxation (μSR) measurements on x=0, 0.1 and 1.0 to investigate the microscopic magnetism. Magnetic ordering has been observed in x=0, 0.1 and 1.0. Furthermore, the ZF-μSR spectra show clear frequency oscillations in x=1.0, indicating a well-defined internal field at the muon site.

Original language	English
Pages (from-to)	e575-e576
Journal	Journal of Magnetism and Magnetic Materials
Volume	310
Issue number	2 SUPPL. PART 2
DOIs	https://doi.org/10.1016/j.jmmm.2006.10.540
Publication status	Published - Mar 2007
Externally published	Yes

Keywords

μSR
Antiferromagnetic ordering
Double perovskites
Valence phase transition

ASJC Scopus subject areas

Electronic, Optical and Magnetic Materials
Condensed Matter Physics

Access to Document

10.1016/j.jmmm.2006.10.540

Cite this

@article{949cd4969e054f0bb94d226eb5c852a1,

title = "A μSR study of the valence phase transition in the double perovskites Ba2PrRu1-xIrxO6",

abstract = "The recent bulk studies have revealed the first-order valence phase transition in Ba2PrRu1-xIrxO6 (0.10≤x≤0.25), while the compounds with x=0 and 1 show antiferromagnetic ordering with TN=120 and 71 K, respectively. We have carried out zero-field (ZF) muon spin relaxation (μSR) measurements on x=0, 0.1 and 1.0 to investigate the microscopic magnetism. Magnetic ordering has been observed in x=0, 0.1 and 1.0. Furthermore, the ZF-μSR spectra show clear frequency oscillations in x=1.0, indicating a well-defined internal field at the muon site.",

keywords = "μSR, Antiferromagnetic ordering, Double perovskites, Valence phase transition",

author = "Hillier, \{A. D.\} and Adroja, \{D. T.\} and W. Kockelmann and M. Wakeshima and Y. Izumiyama and Y. Hinatsu and D. Visser and Rainford, \{B. D.\}",

year = "2007",

month = mar,

doi = "10.1016/j.jmmm.2006.10.540",

language = "English",

volume = "310",

pages = "e575--e576",

journal = "Journal of Magnetism and Magnetic Materials",

issn = "0304-8853",

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TY - JOUR

T1 - A μSR study of the valence phase transition in the double perovskites Ba2PrRu1-xIrxO6

AU - Hillier, A. D.

AU - Adroja, D. T.

AU - Kockelmann, W.

AU - Wakeshima, M.

AU - Izumiyama, Y.

AU - Hinatsu, Y.

AU - Visser, D.

AU - Rainford, B. D.

PY - 2007/3

Y1 - 2007/3

N2 - The recent bulk studies have revealed the first-order valence phase transition in Ba2PrRu1-xIrxO6 (0.10≤x≤0.25), while the compounds with x=0 and 1 show antiferromagnetic ordering with TN=120 and 71 K, respectively. We have carried out zero-field (ZF) muon spin relaxation (μSR) measurements on x=0, 0.1 and 1.0 to investigate the microscopic magnetism. Magnetic ordering has been observed in x=0, 0.1 and 1.0. Furthermore, the ZF-μSR spectra show clear frequency oscillations in x=1.0, indicating a well-defined internal field at the muon site.

AB - The recent bulk studies have revealed the first-order valence phase transition in Ba2PrRu1-xIrxO6 (0.10≤x≤0.25), while the compounds with x=0 and 1 show antiferromagnetic ordering with TN=120 and 71 K, respectively. We have carried out zero-field (ZF) muon spin relaxation (μSR) measurements on x=0, 0.1 and 1.0 to investigate the microscopic magnetism. Magnetic ordering has been observed in x=0, 0.1 and 1.0. Furthermore, the ZF-μSR spectra show clear frequency oscillations in x=1.0, indicating a well-defined internal field at the muon site.

KW - μSR

KW - Antiferromagnetic ordering

KW - Double perovskites

KW - Valence phase transition

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DO - 10.1016/j.jmmm.2006.10.540

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JO - Journal of Magnetism and Magnetic Materials

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IS - 2 SUPPL. PART 2

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